Dimensional study of the dynamical arrest in a random Lorentz gas.
Abstract
The random Lorentz gas (RLG) is a minimal model for transport in heterogeneous media.
Upon increasing the obstacle density, it exhibits a growing subdiffusive transport
regime and then a dynamical arrest. Here, we study the dimensional dependence of the
dynamical arrest, which can be mapped onto the void percolation transition for Poisson-distributed
point obstacles. We numerically determine the arrest in dimensions d=2-6. Comparison
of the results with standard mode-coupling theory reveals that the dynamical theory
prediction grows increasingly worse with d. In an effort to clarify the origin of
this discrepancy, we relate the dynamical arrest in the RLG to the dynamic glass transition
of the infinite-range Mari-Kurchan-model glass former. Through a mixed static and
dynamical analysis, we then extract an improved dimensional scaling form as well as
a geometrical upper bound for the arrest. The results suggest that understanding the
asymptotic behavior of the random Lorentz gas may be key to surmounting fundamental
difficulties with the mode-coupling theory of glasses.
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https://hdl.handle.net/10161/12620Published Version (Please cite this version)
10.1103/PhysRevE.91.042313Publication Info
Jin, Yuliang; & Charbonneau, Patrick (2015). Dimensional study of the dynamical arrest in a random Lorentz gas. Phys Rev E Stat Nonlin Soft Matter Phys, 91(4). pp. 042313. 10.1103/PhysRevE.91.042313. Retrieved from https://hdl.handle.net/10161/12620.This is constructed from limited available data and may be imprecise. To cite this
article, please review & use the official citation provided by the journal.
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Show full item recordScholars@Duke
Patrick Charbonneau
Professor of Chemistry
Professor Charbonneau studies soft matter. His work combines theory and simulation
to understand the glass problem, protein crystallization, microphase formation, and colloidal
assembly in external fields.

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