RIR-MAPLE deposition of plasmonic silver nanoparticles
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© 2016, Springer-Verlag Berlin Heidelberg.Nanoparticles are being explored in many different applications due to the unique properties offered by quantum effects. To broaden the scope of these applications, the deposition of nanoparticles onto substrates in a simple and controlled way is highly desired. In this study, we use resonant infrared matrix-assisted pulsed laser evaporation (RIR-MAPLE) for the deposition of metallic, silver nanoparticles for plasmonic applications. We find that RIR-MAPLE, a simple and versatile approach, is able to deposit silver nanoparticles as large as 80 nm onto different substrates with good adhesion, regardless of substrate properties. In addition, the nanoparticle surface coverage of the substrates, which result from the random distribution of nanoparticles across the substrate per laser pulse, can be simply and precisely controlled by RIR-MAPLE. Polymer films of poly(3-hexylthiophene-2,5-diyl) (P3HT) are also deposited by RIR-MAPLE on top of the deposited silver nanoparticles in order to demonstrate enhanced absorption due to the localized surface plasmon resonance effect. The reported features of RIR-MAPLE nanoparticle deposition indicate that this tool can enable efficient processing of nanoparticle thin films for applications that require specific substrates or configurations that are not easily achieved using solution-based approaches.
Published Version (Please cite this version)10.1007/s00339-016-0360-9
Publication InfoGe, W; Hoang, TB; Mikkelsen, MH; & Stiff-Roberts, Adrienne (2016). RIR-MAPLE deposition of plasmonic silver nanoparticles. Applied Physics A: Materials Science and Processing, 122(9). 10.1007/s00339-016-0360-9. Retrieved from http://hdl.handle.net/10161/12736.
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Professor of Electrical and Computer Engineering
Dr. Stiff-Roberts received both the B.S. degree in physics from Spelman College and the B.E.E. degree in electrical engineering from the Georgia Institute of Technology in 1999. She received an M.S.E. in electrical engineering and a Ph.D. in applied physics in 2001 and 2004, respectively, from the University of Michigan, Ann Arbor, where she investigated high-temperature quantum dot infrared photodetectors grown by molecular beam epitaxy. Dr. Stiff-Roberts joined Duke University in August 2004,