Growing timescales and lengthscales characterizing vibrations of amorphous solids.
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Low-temperature properties of crystalline solids can be understood using harmonic perturbations around a perfect lattice, as in Debye's theory. Low-temperature properties of amorphous solids, however, strongly depart from such descriptions, displaying enhanced transport, activated slow dynamics across energy barriers, excess vibrational modes with respect to Debye's theory (i.e., a boson peak), and complex irreversible responses to small mechanical deformations. These experimental observations indirectly suggest that the dynamics of amorphous solids becomes anomalous at low temperatures. Here, we present direct numerical evidence that vibrations change nature at a well-defined location deep inside the glass phase of a simple glass former. We provide a real-space description of this transition and of the rapidly growing time- and lengthscales that accompany it. Our results provide the seed for a universal understanding of low-temperature glass anomalies within the theoretical framework of the recently discovered Gardner phase transition.
Published Version (Please cite this version)10.1073/pnas.1607730113
Publication InfoBerthier, Ludovic; Charbonneau, Patrick; Jin, Y; Parisi, G; Seoane, B; & Zamponi, Francesco (2016). Growing timescales and lengthscales characterizing vibrations of amorphous solids. Proc Natl Acad Sci U S A, 113(30). pp. 8397-8401. 10.1073/pnas.1607730113. Retrieved from https://hdl.handle.net/10161/15332.
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Associate Professor of Chemistry
Professor Charbonneau studies soft matter. His work combines theory and simulation to understand the glass problem, protein crystallization, microphase formation, and colloidal assembly in external fields.