Dimensional study of the dynamical arrest in a random Lorentz gas.

dc.contributor.author

Jin, Yuliang

dc.contributor.author

Charbonneau, Patrick

dc.coverage.spatial

United States

dc.date.accessioned

2016-08-03T15:53:16Z

dc.date.issued

2015-04

dc.description.abstract

The random Lorentz gas (RLG) is a minimal model for transport in heterogeneous media. Upon increasing the obstacle density, it exhibits a growing subdiffusive transport regime and then a dynamical arrest. Here, we study the dimensional dependence of the dynamical arrest, which can be mapped onto the void percolation transition for Poisson-distributed point obstacles. We numerically determine the arrest in dimensions d=2-6. Comparison of the results with standard mode-coupling theory reveals that the dynamical theory prediction grows increasingly worse with d. In an effort to clarify the origin of this discrepancy, we relate the dynamical arrest in the RLG to the dynamic glass transition of the infinite-range Mari-Kurchan-model glass former. Through a mixed static and dynamical analysis, we then extract an improved dimensional scaling form as well as a geometrical upper bound for the arrest. The results suggest that understanding the asymptotic behavior of the random Lorentz gas may be key to surmounting fundamental difficulties with the mode-coupling theory of glasses.

dc.identifier

http://www.ncbi.nlm.nih.gov/pubmed/25974497

dc.identifier.eissn

1550-2376

dc.identifier.uri

https://hdl.handle.net/10161/12620

dc.language

eng

dc.publisher

American Physical Society (APS)

dc.relation.ispartof

Phys Rev E Stat Nonlin Soft Matter Phys

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10.1103/PhysRevE.91.042313

dc.subject

Gases

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Glass

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Hydrodynamics

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Models, Theoretical

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Phase Transition

dc.title

Dimensional study of the dynamical arrest in a random Lorentz gas.

dc.type

Journal article

duke.contributor.orcid

Charbonneau, Patrick|0000-0001-7174-0821

pubs.author-url

http://www.ncbi.nlm.nih.gov/pubmed/25974497

pubs.begin-page

042313

pubs.issue

4

pubs.organisational-group

Chemistry

pubs.organisational-group

Duke

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Physics

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Trinity College of Arts & Sciences

pubs.publication-status

Published

pubs.volume

91

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